Condensed Matter, abstract
cond-mat/0409269

From: D. R. Hamann [view email]
Date: Fri, 10 Sep 2004 14:51:30 GMT   (316kb)

Metric Tensor Formulation of Strain in Density-Functional Perturbation Theory

Authors: D. R. Hamann, (1,2,3) Xifan Wu, (1) Karin M. Rabe (1), David Vanderbilt (1) ((1)Department of Physics and Astronomy, Rutgers University, Piscataway, NJ, (2)Bell Laboratories, Lucent Technologies, Murray Hill, NJ, (3)Mat-Sim Research LLC, Murray Hill, NJ)
Comments: 25 pages, no figures, submitted to Phys. Rev. B
Subj-class: Materials Science; Other
The direct calculation of the elastic and piezoelectric tensors of solids can be accomplished by treating homogeneous strain within the framework of density-functional perturbation theory. By formulating the energy functional in reduced coordinates, we show that the strain perturbation enters only through metric tensors, and can be treated in a manner exactly paralleling the treatment of other perturbations. We present an analysis of the strain perturbation of the plane-wave pseudopotential functional, including the internal strain terms necessary to treat the atomic-relaxation contributions. Procedures for computationally verifying these expressions by comparison with numerical derivatives of ground-state calculations are described and illustrated.

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